This is what I used to enlarge the MPS manually:
for bond in 1:(length(ψ₀)-1)
bond_index = commonind(ψ₀[bond], ψ₀[bond + 1])
aux = Index(new_dim; tags=tags(bond_index))
ψ₀[bond] = ψ₀[bond] * delta(bond_index, aux)
ψ₀[bond + 1] = ψ₀[bond + 1] * delta(bond_index, aux)
end
You could plug it in your code just after you create the MPS.